WO2003088374A3 - Asymmetric supercapacitor device with extended capability - Google Patents

Asymmetric supercapacitor device with extended capability Download PDF

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Publication number
WO2003088374A3
WO2003088374A3 PCT/CA2003/000508 CA0300508W WO03088374A3 WO 2003088374 A3 WO2003088374 A3 WO 2003088374A3 CA 0300508 W CA0300508 W CA 0300508W WO 03088374 A3 WO03088374 A3 WO 03088374A3
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WO
WIPO (PCT)
Prior art keywords
chosen
group
carbon
separator
oxide
Prior art date
Application number
PCT/CA2003/000508
Other languages
French (fr)
Other versions
WO2003088374A2 (en
Inventor
Jeffrey Philips
Donald Hewson
Original Assignee
Powergenix Systems Inc
Jeffrey Philips
Donald Hewson
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Powergenix Systems Inc, Jeffrey Philips, Donald Hewson filed Critical Powergenix Systems Inc
Priority to AU2003227150A priority Critical patent/AU2003227150A1/en
Publication of WO2003088374A2 publication Critical patent/WO2003088374A2/en
Publication of WO2003088374A3 publication Critical patent/WO2003088374A3/en

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Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01G—CAPACITORS; CAPACITORS, RECTIFIERS, DETECTORS, SWITCHING DEVICES OR LIGHT-SENSITIVE DEVICES, OF THE ELECTROLYTIC TYPE
    • H01G9/00—Electrolytic capacitors, rectifiers, detectors, switching devices, light-sensitive or temperature-sensitive devices; Processes of their manufacture
    • H01G9/22—Devices using combined reduction and oxidation, e.g. redox arrangement or solion
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01G—CAPACITORS; CAPACITORS, RECTIFIERS, DETECTORS, SWITCHING DEVICES OR LIGHT-SENSITIVE DEVICES, OF THE ELECTROLYTIC TYPE
    • H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
    • H01G11/02—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof using combined reduction-oxidation reactions, e.g. redox arrangement or solion
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01G—CAPACITORS; CAPACITORS, RECTIFIERS, DETECTORS, SWITCHING DEVICES OR LIGHT-SENSITIVE DEVICES, OF THE ELECTROLYTIC TYPE
    • H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
    • H01G11/04—Hybrid capacitors
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01G—CAPACITORS; CAPACITORS, RECTIFIERS, DETECTORS, SWITCHING DEVICES OR LIGHT-SENSITIVE DEVICES, OF THE ELECTROLYTIC TYPE
    • H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
    • H01G11/22—Electrodes
    • H01G11/30—Electrodes characterised by their material
    • H01G11/46—Metal oxides
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01G—CAPACITORS; CAPACITORS, RECTIFIERS, DETECTORS, SWITCHING DEVICES OR LIGHT-SENSITIVE DEVICES, OF THE ELECTROLYTIC TYPE
    • H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
    • H01G11/52—Separators
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/24—Alkaline accumulators
    • H01M10/30—Nickel accumulators
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/04—Processes of manufacture in general
    • H01M4/0438—Processes of manufacture in general by electrochemical processing
    • H01M4/045—Electrochemical coating; Electrochemical impregnation
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/24—Electrodes for alkaline accumulators
    • H01M4/32—Nickel oxide or hydroxide electrodes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/52—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of nickel, cobalt or iron
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/58—Selection of substances as active materials, active masses, active liquids of inorganic compounds other than oxides or hydroxides, e.g. sulfides, selenides, tellurides, halogenides or LiCoFy; of polyanionic structures, e.g. phosphates, silicates or borates
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M50/00—Constructional details or processes of manufacture of the non-active parts of electrochemical cells other than fuel cells, e.g. hybrid cells
    • H01M50/40—Separators; Membranes; Diaphragms; Spacing elements inside cells
    • H01M50/409—Separators, membranes or diaphragms characterised by the material
    • H01M50/411—Organic material
    • H01M50/414—Synthetic resins, e.g. thermoplastics or thermosetting resins
    • H01M50/417—Polyolefins
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M50/00—Constructional details or processes of manufacture of the non-active parts of electrochemical cells other than fuel cells, e.g. hybrid cells
    • H01M50/40—Separators; Membranes; Diaphragms; Spacing elements inside cells
    • H01M50/409—Separators, membranes or diaphragms characterised by the material
    • H01M50/411—Organic material
    • H01M50/414—Synthetic resins, e.g. thermoplastics or thermosetting resins
    • H01M50/423—Polyamide resins
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M50/00—Constructional details or processes of manufacture of the non-active parts of electrochemical cells other than fuel cells, e.g. hybrid cells
    • H01M50/40—Separators; Membranes; Diaphragms; Spacing elements inside cells
    • H01M50/409—Separators, membranes or diaphragms characterised by the material
    • H01M50/44—Fibrous material
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01G—CAPACITORS; CAPACITORS, RECTIFIERS, DETECTORS, SWITCHING DEVICES OR LIGHT-SENSITIVE DEVICES, OF THE ELECTROLYTIC TYPE
    • H01G11/00—Hybrid capacitors, i.e. capacitors having different positive and negative electrodes; Electric double-layer [EDL] capacitors; Processes for the manufacture thereof or of parts thereof
    • H01G11/22—Electrodes
    • H01G11/24—Electrodes characterised by structural features of the materials making up or comprised in the electrodes, e.g. form, surface area or porosity; characterised by the structural features of powders or particles used therefor
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/04—Construction or manufacture in general
    • H01M10/0472—Vertically superposed cells with vertically disposed plates
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M2004/026—Electrodes composed of, or comprising, active material characterised by the polarity
    • H01M2004/028—Positive electrodes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/04—Processes of manufacture in general
    • H01M4/0402—Methods of deposition of the material
    • H01M4/0404—Methods of deposition of the material by coating on electrode collectors
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/04—Processes of manufacture in general
    • H01M4/049—Manufacturing of an active layer by chemical means
    • H01M4/0497—Chemical precipitation
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/64—Carriers or collectors
    • H01M4/66—Selection of materials
    • H01M4/661—Metal or alloys, e.g. alloy coatings
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/64—Carriers or collectors
    • H01M4/70—Carriers or collectors characterised by shape or form
    • H01M4/80—Porous plates, e.g. sintered carriers
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10—Energy storage using batteries
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/13—Energy storage using capacitors
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

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  • Engineering & Computer Science (AREA)
  • Power Engineering (AREA)
  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Microelectronics & Electronic Packaging (AREA)
  • General Chemical & Material Sciences (AREA)
  • Electrochemistry (AREA)
  • Materials Engineering (AREA)
  • Inorganic Chemistry (AREA)
  • Manufacturing & Machinery (AREA)
  • Battery Electrode And Active Subsutance (AREA)
  • Cell Electrode Carriers And Collectors (AREA)
  • Cell Separators (AREA)

Abstract

An energy storage device has a nickel-based positive electrode, a carbon-based negative electrode, a separator, and an aqueous electrolyte. The positive electrode comprises from 3% to 95% by weight of nickel hydroxide, with the balance being chosen from the group consisting of: nickel powder, cobalt powder, carbon powder, and mixtures thereof. The negative electrode comprises from 10% to 95% by weight of carbon, with the balance being at least one redox couple. The electrolyte is an aqueous alkaline solution, and the separator is chosen from the group consisting of: non-woven nylon separator material, microporous polypropylene, microporous polyethylene, and combinations and mixtures thereof. Typically, the redox couple is chosen from the group of active redox couples which include, as their active material, bismuth oxide, indium oxide, cobalt oxide, iron oxide, iron hydroxide, hydrides of metals from the Groups IIIA, IIIB, IVA, IVB, VB, VIB, VIIB, and VIII, of the Periodic Table, hydrides of mischmetals, oxides of mischmetals, and combinations thereof.
PCT/CA2003/000508 2002-04-08 2003-04-04 Asymmetric supercapacitor device with extended capability WO2003088374A2 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
AU2003227150A AU2003227150A1 (en) 2002-04-08 2003-04-04 Asymmetric supercapacitor device with extended capability

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CA002380954A CA2380954A1 (en) 2002-04-08 2002-04-08 Supercapacitor device with extended capability
CA2,380,954 2002-04-08

Publications (2)

Publication Number Publication Date
WO2003088374A2 WO2003088374A2 (en) 2003-10-23
WO2003088374A3 true WO2003088374A3 (en) 2004-09-02

Family

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PCT/CA2003/000508 WO2003088374A2 (en) 2002-04-08 2003-04-04 Asymmetric supercapacitor device with extended capability

Country Status (3)

Country Link
AU (1) AU2003227150A1 (en)
CA (1) CA2380954A1 (en)
WO (1) WO2003088374A2 (en)

Families Citing this family (10)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CA2380954A1 (en) * 2002-04-08 2003-10-08 Powergenix Systems, Inc. Supercapacitor device with extended capability
CN102354617B (en) * 2011-09-30 2012-10-03 天津国泰之光新材料技术研究院有限公司 Positive plate slurry of high-energy nickel/carbon super capacitor
CN102354615B (en) * 2011-09-30 2013-01-16 天津国泰之光新材料技术研究院有限公司 Preparation method of slurry for positive plate of high-energy nickel-carbon supercapacitor
FR2989215B1 (en) * 2012-04-06 2015-04-03 Thales Sa HYBRID ELECTRODE FOR SUPERCONDENSER
EP3435449B1 (en) * 2014-07-09 2019-09-04 VARTA Microbattery GmbH Secondary electrochemical cell
EP2966709B1 (en) * 2014-07-09 2018-01-10 VARTA Microbattery GmbH Secondary electrochemical element
EP3178125B1 (en) * 2014-08-08 2018-09-26 VARTA Microbattery GmbH Secondary electrochemical element based on nickel / iron
EP2983236B1 (en) * 2014-08-08 2017-10-18 VARTA Microbattery GmbH Secondary electrochemical element based on nickel/iron
CN104681888B (en) * 2015-01-06 2017-02-22 宁波中车新能源科技有限公司 Negative-pressure stepped formation method of lithium ion capacitance battery
CN109950050B (en) * 2019-04-17 2021-04-16 武汉工程大学 Preparation method of supercapacitor electrode material based on carbonized melamine foam @ Bi2O3 nanosheets

Citations (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US5585999A (en) * 1994-09-30 1996-12-17 The United States Of America As Represented By The Secretary Of The Air Force Supercapacitor electrochemical cell
EP0786786A1 (en) * 1995-08-14 1997-07-30 Aktsionernoe Obschestvo Zakrytogo Tipa "Elton" Capacitor with a double electrical layer
EP0964416A1 (en) * 1997-11-11 1999-12-15 Nauchno-Proizvodstvennoe Predpriyatie "EKSIN" Capacitor with dual electric layer
US6181546B1 (en) * 1999-01-19 2001-01-30 Aktsionernoe Obschestvo Zakrytogo Tipa “Elton” Double layer capacitor
WO2001057895A1 (en) * 2000-02-01 2001-08-09 Cabot Corporation Capacitors and supercapacitors containing modified carbon products
EP1156500A1 (en) * 1998-11-27 2001-11-21 Sergey Nikolaevich Razumov Asymmetric electrochemical capacitor
CA2380954A1 (en) * 2002-04-08 2003-10-08 Powergenix Systems, Inc. Supercapacitor device with extended capability

Patent Citations (8)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US5585999A (en) * 1994-09-30 1996-12-17 The United States Of America As Represented By The Secretary Of The Air Force Supercapacitor electrochemical cell
EP0786786A1 (en) * 1995-08-14 1997-07-30 Aktsionernoe Obschestvo Zakrytogo Tipa "Elton" Capacitor with a double electrical layer
US5986876A (en) * 1995-08-14 1999-11-16 Aktsionernoe Obschestvo Zakrytogo Tipa "Elton" Double-layer capacitor
EP0964416A1 (en) * 1997-11-11 1999-12-15 Nauchno-Proizvodstvennoe Predpriyatie "EKSIN" Capacitor with dual electric layer
EP1156500A1 (en) * 1998-11-27 2001-11-21 Sergey Nikolaevich Razumov Asymmetric electrochemical capacitor
US6181546B1 (en) * 1999-01-19 2001-01-30 Aktsionernoe Obschestvo Zakrytogo Tipa “Elton” Double layer capacitor
WO2001057895A1 (en) * 2000-02-01 2001-08-09 Cabot Corporation Capacitors and supercapacitors containing modified carbon products
CA2380954A1 (en) * 2002-04-08 2003-10-08 Powergenix Systems, Inc. Supercapacitor device with extended capability

Non-Patent Citations (2)

* Cited by examiner, † Cited by third party
Title
CONWAY B E ET AL: "The role and utilization of pseudocapacitance for energy storage by supercapacitors", JOURNAL OF POWER SOURCES, ELSEVIER SEQUOIA S.A. LAUSANNE, CH, vol. 66, no. 1-2, 1 May 1997 (1997-05-01), pages 1 - 14, XP004082296, ISSN: 0378-7753 *
CONWAY B E: "Transition from 'supercapacitor' to 'battery' behavior in electrochemical energy storage", PROCEEDINGS OF THE INTERNATIONAL POWER SOURCES SYMPOSIUM. CHERRY HILL, JUNE 25 - 28, 1990, NEW YORK, IEEE, US, vol. SYMP. 34, 25 June 1990 (1990-06-25), pages 319 - 327, XP010038403, ISBN: 0-87942-604-7 *

Also Published As

Publication number Publication date
AU2003227150A8 (en) 2003-10-27
CA2380954A1 (en) 2003-10-08
WO2003088374A2 (en) 2003-10-23
AU2003227150A1 (en) 2003-10-27

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